Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

  • Letter
  • Published:

Maximal spontaneous photon emission and energy loss from free electrons

Subjects

A Publisher Correction to this article was published on 23 July 2018

This article has been updated

Abstract

Free-electron radiation such as Cerenkov1, Smith–Purcell2 and transition radiation3,4 can be greatly affected by structured optical environments, as has been demonstrated in a variety of polaritonic5,6, photonic-crystal7 and metamaterial8,9,10 systems. However, the amount of radiation that can ultimately be extracted from free electrons near an arbitrary material structure has remained elusive. Here we derive a fundamental upper limit to the spontaneous photon emission and energy loss of free electrons, regardless of geometry, which illuminates the effects of material properties and electron velocities. We obtain experimental evidence for our theory with quantitative measurements of Smith–Purcell radiation. Our framework allows us to make two predictions. One is a new regime of radiation operation—at subwavelength separations, slower (non-relativistic) electrons can achieve stronger radiation than fast (relativistic) electrons. The other is a divergence of the emission probability in the limit of lossless materials. We further reveal that such divergences can be approached by coupling free electrons to photonic bound states in the continuum11,12,13. Our findings suggest that compact and efficient free-electron radiation sources from microwaves to the soft X-ray regime may be achievable without requiring ultrahigh accelerating voltages.

This is a preview of subscription content, access via your institution

Access options

Buy this article

Prices may be subject to local taxes which are calculated during checkout

Fig. 1: Theoretical framework and predictions.
Fig. 2: Optimal electron velocities for maximal Smith–Purcell radiation.
Fig. 3: Experimental probing of the upper limit.
Fig. 4: Strong enhancement of Smith–Purcell radiation via high-Q resonances near a photonic BIC.

Similar content being viewed by others

Change history

  • 23 July 2018

    In the version of this Letter originally published, an older version of the Supplementary Information was uploaded by mistake, in which the notation did not match the main text. This has been corrected.

References

  1. Cherenkov, P. A. Visible glow under exposure of gamma radiation. Dokl. Akad. Nauk SSSR 2, 451–454 (1934).

    Google Scholar 

  2. Smith, S. J. & Purcell, E. Visible light from localized surface charges moving across a grating. Phys. Rev. 92, 1069 (1953).

    Article  ADS  Google Scholar 

  3. Ginsburg, V. & Frank, I. Radiation of a uniformly moving electron due to its transition from one medium into another. Zh. Eksp. Teor. Fiz. 16, 15–28 (1946).

    Google Scholar 

  4. Goldsmith, P. & Jelley, J. Optical transition radiation from protons entering metal surfaces. Philos. Mag. 4, 836–844 (1959).

    Article  ADS  Google Scholar 

  5. Liu, S. et al. Surface polariton Cherenkov light radiation source. Phys. Rev. Lett. 109, 153902 (2012).

    Article  ADS  Google Scholar 

  6. Kaminer, I. et al. Efficient plasmonic emission by the quantum Čerenkov effect from hot carriers in graphene. Nat. Commun. 7, ncomms11880 (2016).

    Article  ADS  Google Scholar 

  7. Luo, C., Ibanescu, M., Johnson, S. G. & Joannopoulos, J. Cerenkov radiation in photonic crystals. Science 299, 368–371 (2003).

    Article  ADS  Google Scholar 

  8. Adamo, G. et al. Light well: a tunable free-electron light source on a chip. Phys. Rev. Lett. 103, 113901 (2009).

    Article  ADS  Google Scholar 

  9. Ginis, V., Danckaert, J., Veretennicoff, I. & Tassin, P. Controlling Cherenkov radiation with transformation-optical metamaterials. Phys. Rev. Lett. 113, 167402 (2014).

    Article  ADS  Google Scholar 

  10. Liu, F. et al. Integrated Cherenkov radiation emitter eliminating the electron velocity threshold. Nat. Photon. 11, 289–292 (2017).

    Article  ADS  Google Scholar 

  11. Hsu, C. W. et al. Observation of trapped light within the radiation continuum. Nature 499, 188–191, (2013).

    Article  ADS  Google Scholar 

  12. Yang, Y., Peng, C., Liang, Y., Li, Z. & Noda, S. Analytical perspective for bound states in the continuum in photonic crystal slabs. Phys. Rev. Lett. 113, 037401 (2014).

    Article  ADS  Google Scholar 

  13. Hsu, C. W., Zhen, B., Stone, A. D., Joannopoulos, J. D. & Soljacic, M. Bound states in the continuum. Nat. Rev. Mater. 1, 16048 (2016).

    Article  ADS  Google Scholar 

  14. Urata, J. et al. Superradiant Smith–Purcell emission. Phys. Rev. Lett. 80, 516–519 (1998).

    Article  ADS  Google Scholar 

  15. Korbly, S., Kesar, A., Sirigiri, J. & Temkin, R. Observation of frequency-locked coherent terahertz Smith-Purcell radiation. Phys. Rev. Lett. 94, 054803 (2005).

    Article  ADS  Google Scholar 

  16. Doucas, G., Mulvey, J., Omori, M., Walsh, J. & Kimmitt, M. First observation of Smith-Purcell radiation from relativistic electrons. Phys. Rev. Lett. 69, 1761–1764 (1992).

    Article  ADS  Google Scholar 

  17. Kube, G. et al. Observation of optical Smith-Purcell radiation at an electron beam energy of 855 MeV. Phys. Rev. E 65, 056501 (2002).

    Article  ADS  Google Scholar 

  18. Yamamoto, N., de Abajo, F. J. G. & Myroshnychenko, V. Interference of surface plasmons and Smith-Purcell emission probed by angle-resolved cathodoluminescence spectroscopy. Phys. Rev. B 91, 125144 (2015).

    Article  ADS  Google Scholar 

  19. Kaminer, I. et al. Spectrally and spatially resolved Smith-Purcell radiation in plasmonic crystals with short-range disorder. Phys. Rev. X 7, 011003 (2017).

    Google Scholar 

  20. Moran, M. J. X-ray generation by the Smith-Purcell effect. Phys. Rev. Lett. 69, 2523–2526 (1992).

    Article  ADS  Google Scholar 

  21. van den Berg, P. Smith-Purcell radiation from a point charge moving parallel to a reflection grating. J. Opt. Soc. Am. 63, 1588–1597 (1973).

    Article  ADS  Google Scholar 

  22. Haeberlé, O., Rullhusen, P., Salomé, J.-M. & Maene, N. Calculations of Smith-Purcell radiation generated by electrons of 1–100 MeV. Phys. Rev. E 49, 3340–3352 (1994).

    Article  ADS  Google Scholar 

  23. Sergeeva, D. Y., Tishchenko, A. & Strikhanov, M. Conical diffraction effect in optical and x-ray Smith-Purcell radiation. Phys. Rev. ST Accel. Beams 18, 052801 (2015).

    Article  ADS  Google Scholar 

  24. Pendry, J. & Martin-Moreno, L. Energy loss by charged particles in complex media. Phys. Rev. B 50, 5062–5073 (1994).

    Article  ADS  Google Scholar 

  25. García de Abajo, F. J. Smith-Purcell radiation emission in aligned nanoparticles. Phys. Rev. E 61, 5743–5752 (2000).

    Article  ADS  Google Scholar 

  26. García de Abajo, F. J. Optical excitations in electron microscopy. Rev. Mod. Phys. 82, 209–275 (2010).

    Article  ADS  Google Scholar 

  27. Miller, O. D. et al. Fundamental limits to optical response in absorptive systems. Opt. Express 24, 3329–3364 (2016).

    Article  ADS  Google Scholar 

  28. Yang, Y., Miller, O. D., Christensen, T., Joannopoulos, J. D. & Soljačić, M. Low-loss plasmonic dielectric nanoresonators. Nano Lett. 17, 3238–3245 (2017).

    Article  ADS  Google Scholar 

  29. Miller, O. D., Johnson, S. G. & Rodriguez, A. W. Shape-independent limits to near-field radiative heat transfer. Phys. Rev. Lett. 115, 204302 (2015).

    Article  ADS  Google Scholar 

  30. Friedman, A., Gover, A., Kurizki, G., Ruschin, S. & Yariv, A. Spontaneous and stimulated emission from quasifree electrons. Rev. Mod. Phys. 60, 471–535 (1988).

    Article  ADS  Google Scholar 

  31. Massuda, A. et al. Preprint at https://arxiv.org/abs/1710.05358 (2017).

  32. Gradshteyn, I. S. & Ryzhik, I. M. in Tables of Integrals, Series, and Products 6th edn (eds Jeffrey, A. & Zwillinger, D.) 843–850 and 1022–1025 (Academic, San Diego, CA, 2000).

  33. Pendry, J., Martin-Moreno, L. & Garcia-Vidal, F. Mimicking surface plasmons with structured surfaces. Science 305, 847–848 (2004).

    Article  ADS  Google Scholar 

  34. Andrews, H. L. & Brau, C. A. Gain of a Smith-Purcell free-electron laser. Phys. Rev. ST Accel. Beams 7, 070701 (2004).

    Article  ADS  Google Scholar 

  35. Kumar, V. & Kim, K.-J. Analysis of Smith-Purcell free-electron lasers. Phys. Rev. E 73, 026501 (2006).

    Article  ADS  Google Scholar 

  36. Green, M. A. Self-consistent optical parameters of intrinsic silicon at 300 K including temperature coefficients. Sol. Energy Mater. Sol. Cells 92, 1305–1310 (2008).

    Article  Google Scholar 

  37. Schächter, L. & Ron, A. Smith-Purcell free-electron laser. Phys. Rev. A 40, 876–896 (1989).

    Article  ADS  Google Scholar 

  38. Peralta, E. A. et al. Demonstration of electron acceleration in a laser-driven dielectric microstructure. Nature 503, 91–94 (2013).

    Article  ADS  Google Scholar 

  39. Breuer, J. & Hommelhoff, P. Laser-based acceleration of nonrelativistic electrons at a dielectric structure. Phys. Rev. Lett. 111, 134803 (2013).

    Article  ADS  Google Scholar 

  40. Palik, E. D. Handbook of Optical Constants of Solids Vol. 3 (Academic, San Diego, CA, 1998).

Download references

Acknowledgements

The authors acknowledge fruitful discussions with K. Berggren, S. Yang, C. Peng, A. Gover, B. Zhen, L. J. Wong, X. Lin, D. Zhu, Yu. Yang, T. Dubcek and N. Rivera. We thank P. Rebusco for critical reading and editing of the manuscript. This work was performed in part at the Harvard University Center for Nanoscale Systems (CNS), a member of the National Nanotechnology Coordinated Infrastructure Network (NNCI), which is supported by the National Science Foundation under NSF ECCS award no. 1541959. This work was partly supported by the Army Research Office through the Institute for Soldier Nanotechnologies under contract nos W911NF-18-2-0048 and W911NF-13-D-0001. Y.Y. was partly supported by the MRSEC Program of the National Science Foundation under grant no. DMR-1419807. T.C. was supported by the Danish Council for Independent Research (grant no. DFFC6108-00667). O.D.M. was supported by the Air Force Office of Scientific Research under award no. FA9550-17-1-0093. I.K. was partially supported by the Azrieli foundation and the Seventh Framework Programme of the European Research Council (FP7- Marie Curie IOF) under grant agreement no. 328853CMC-BSiCS.

Author information

Authors and Affiliations

Authors

Contributions

Y.Y., O.D.M., I.K. and M.S. conceived the project. Y.Y. developed the analytical models and numerical calculations. A.M. prepared the sample under study. Y.Y., A.M., C.R.-C., S.E.K. and I.K. performed the experiment. Y.Y., T.C. and O.D.M. analysed the asymptotics and bulk loss of the limit. S.G.J., J.D.J., O.D.M., I.K. and M.S. supervised the project. Y.Y. wrote the manuscript with input from all authors.

Corresponding authors

Correspondence to Yi Yang, Owen D. Miller or Ido Kaminer.

Ethics declarations

Competing interests

The authors declare no competing interests.

Additional information

Publisher’s note: Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Supplementary information

Supplementary Information

10 Figure, 12 References

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Yang, Y., Massuda, A., Roques-Carmes, C. et al. Maximal spontaneous photon emission and energy loss from free electrons. Nature Phys 14, 894–899 (2018). https://doi.org/10.1038/s41567-018-0180-2

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1038/s41567-018-0180-2

This article is cited by

Search

Quick links

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing