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Elastic films of single-crystal two-dimensional covalent organic frameworks
- Yonghang Yang
- , Baokun Liang
- & Zhikun Zheng
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Article
| Open AccessForce-controlled release of small molecules with a rotaxane actuator
A rotaxane-based mechanochemical system enables force-controlled release of multiple cargo molecules that are appended to its molecular axle.
- Lei Chen
- , Robert Nixon
- & Guillaume De Bo
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High fatigue resistance in a titanium alloy via near-void-free 3D printing
We successfully rebuild an approximate void-free additive manufacturing microstructure in Ti-6Al-4V titanium alloy by the development of a void-free additive manufacturing processing technique through an understanding of the asynchronism of phase transformation and grain growth.
- Zhan Qu
- , Zhenjun Zhang
- & Zhefeng Zhang
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Article
| Open AccessTwisted-layer boron nitride ceramic with high deformability and strength
A bulk ceramic composed of interlocked boron nitride nanoplates with a laminated structure of twist-stacked nanoslices is created using hot-pressing and spark plasma sintering, which exhibits large elastic and plastic deformability and high strength at room temperature.
- Yingju Wu
- , Yang Zhang
- & Yongjun Tian
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Negative mixing enthalpy solid solutions deliver high strength and ductility
A HfNbTiVAl10 alloy shows tensile ductility and ultrahigh yield strength from the addition of aluminium to a HfNbTiV alloy, resulting in a negative mixing enthalpy solid solution, which promotes strength and favours formation of hierarchical chemical fluctuations.
- Zibing An
- , Ang Li
- & Xiaodong Han
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Structural transition and migration of incoherent twin boundary in diamond
We report atomic observations of six incoherent twin boundary configurations and structural transitions in diamond at room temperature, showing a dislocation-mediated mechanism different from metallic systems and shedding new light on grain boundary behaviour.
- Ke Tong
- , Xiang Zhang
- & Yongjun Tian
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Multiscale stress deconcentration amplifies fatigue resistance of rubber
A rubber in which highly entangled long polymers strongly adhere with rigid particles deconcentrates stress across multiple scales, amplifying the fatigue threshold.
- Jason Steck
- , Junsoo Kim
- & Zhigang Suo
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Dynamic diagnosis of metamaterials through laser-induced vibrational signatures
A high-throughput, non-contact framework is described that uses the laser-induced vibrational signatures of metamaterials to non-destructively quantify their omnidirectional elastic information, dynamic linear properties, damping properties and defects.
- Yun Kai
- , Somayajulu Dhulipala
- & Carlos M. Portela
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Multistable sheets with rewritable patterns for switchable shape-morphing
To demonstrate the power of multistability, a specific class of groovy metasheets is introduced as a new shape-morphing platform that allows repeated switching from the flat state to multiple, precisely selected and stable three-dimensional shapes.
- A. S. Meeussen
- & M. van Hecke
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Article
| Open AccessBonding wood with uncondensed lignins as adhesives
A straightforward strategy for preparing lignin-based wood adhesives from lignocellulosic biomass is described, with the resulting adhesives demonstrating performance attractive for plywood manufacture.
- Guangxu Yang
- , Zhenggang Gong
- & Li Shuai
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Autonomous healing of fatigue cracks via cold welding
We report that fatigue cracks in pure metals can undergo intrinsic self-healing; they were observed to heal by crack flank cold welding induced by local stress state and grain boundary migration.
- Christopher M. Barr
- , Ta Duong
- & Brad L. Boyce
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Organic–inorganic covalent–ionic molecules for elastic ceramic plastic
Covalent organic molecules can be combined with ionic inorganic molecules to create a hybrid material demonstrating paradoxical mechanical properties in a bottom-up manner, enabling the manufacture of an ‘elastic ceramic plastic’.
- Weifeng Fang
- , Zhao Mu
- & Zhaoming Liu
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| Open AccessStrong and ductile titanium–oxygen–iron alloys by additive manufacturing
Combining alloy design with additive manufacturing process design creates α–β titanium–oxygen–iron alloys that are both strong and ductile, with the potential to revitalize off-grade sponge titanium and thereby reduce the carbon footprint of the titanium industry.
- Tingting Song
- , Zibin Chen
- & Ma Qian
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Dynamic crosslinking compatibilizes immiscible mixed plastics
A new compatibilization strategy installs dynamic crosslinkers into several classes of binary, ternary and postconsumer immiscible polymer mixtures in situ, with the resulting compatibilized dynamic thermosets exhibiting intrinsic reprocessability and enhanced tensile strength and creep resistance.
- Ryan W. Clarke
- , Tobias Sandmeier
- & Eugene Y.-X. Chen
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Shape memory in self-adapting colloidal crystals
Preparing crystals held together with macromolecular bonds can create shape memory materials that can be engineered to exhibit a wide range of reversible changes useful for chemical sensing, optics and robotics.
- Seungkyu Lee
- , Heather A. Calcaterra
- & Chad A. Mirkin
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Anomalous slip in body-centred cubic metals
Observations by transmission electron microscopy of deforming niobium and tungsten at low temperature shows that anomalous slip in body-centred cubic metals arises from the unusually high mobility of multi-junctions, which is a source of softening.
- Daniel Caillard
- , Baptiste Bienvenu
- & Emmanuel Clouet
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Strong yet ductile nanolamellar high-entropy alloys by additive manufacturing
An additive manufacturing strategy is used to produce dual-phase nanolamellar high-entropy alloys that show a combination of enhanced high yield strength and high tensile ductility.
- Jie Ren
- , Yin Zhang
- & Wen Chen
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Uniting tensile ductility with ultrahigh strength via composition undulation
A nanocrystalline metallic alloy with ultrahigh tensile strength and good ductility is achieved by introducing compositional undulation in a highly concentrated solid solution.
- Heng Li
- , Hongxiang Zong
- & Jun Sun
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| Open AccessHydrogen trapping and embrittlement in high-strength Al alloys
Atom-scale analysis of hydrogen and other elements at the grain boundaries of a 7xxx aluminium alloy shows that co-segregation of elements favours grain boundary decohesion, and that hydrogen embrittlement is prevented by strong partitioning into the second-phase particles.
- Huan Zhao
- , Poulami Chakraborty
- & Dierk Raabe
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A highly distorted ultraelastic chemically complex Elinvar alloy
A chemically complex alloy that exhibits a high elastic strain limit and low internal friction is described; it also has an Elinvar effect (invariant elastic modulus) over a large temperature range, up to 627 °C.
- Q. F. He
- , J. G. Wang
- & Y. Yang
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Irreversible synthesis of an ultrastrong two-dimensional polymeric material
The solution-phase irreversible synthesis of a two-dimensional polymer with excellent elastic modulus and yield strength is reported.
- Yuwen Zeng
- , Pavlo Gordiichuk
- & Michael S. Strano
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Ultrahard bulk amorphous carbon from collapsed fullerene
Preparing amorphous phases of carbon with mostly sp3 bonding in bulk is challenging, but macroscopic samples that are nearly pure sp3 are synthesized here by heating fullerenes at high pressure.
- Yuchen Shang
- , Zhaodong Liu
- & Bingbing Liu
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An elastic metal–organic crystal with a densely catenated backbone
A rubber-like, metal–organic crystal is reported with a mechanically interlocked catenane backbone, which could allow for easy guest molecule uptake and release.
- Wenjing Meng
- , Shun Kondo
- & Hiroshi Sato
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Perspective |
Mechanical computing
Computing approaches based on mechanical mechanisms are discussed, with a view towards a framework in which adaptable materials and structures act as a distributed information processing network.
- Hiromi Yasuda
- , Philip R. Buskohl
- & Jordan R. Raney
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Structured fabrics with tunable mechanical properties
A structured fabric constructed of linked hollow polyhedral particles (resembling chain mail) can be simply and reversibly tuned between flexible and rigid states; when it is compressed, its linked particles become jammed.
- Yifan Wang
- , Liuchi Li
- & Chiara Daraio
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Extreme flow simulations reveal skeletal adaptations of deep-sea sponges
High-performance hydrodynamic simulations show that the skeletal structure of the deep-sea sponge Euplectella aspergillum reduces the hydrodynamic stresses on it, while possibly being beneficial for feeding and reproduction.
- Giacomo Falcucci
- , Giorgio Amati
- & Sauro Succi
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Bifunctional nanoprecipitates strengthen and ductilize a medium-entropy alloy
Increased strength and ductility in a medium-entropy alloy of Fe, Ni, Al and Ti is demonstrated using nanoprecipitates that simultaneously hinder phase transformation and block dislocation motion.
- Ying Yang
- , Tianyi Chen
- & Easo P. George
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Direct observation of chemical short-range order in a medium-entropy alloy
Direct experimental evidence of chemical short-range atomic-scale ordering (CSRO) in a VCoNi medium-entropy alloy is provided via diffraction and electron microscopy, analysed from specific crystallographic directions.
- Xuefei Chen
- , Qi Wang
- & En Ma
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Multistable inflatable origami structures at the metre scale
Origami-inspired multistable structures that can be inflated from flat to three dimensions have been designed; a library of foldable shapes is created and then combined to build metre-scale functional structures.
- David Melancon
- , Benjamin Gorissen
- & Katia Bertoldi
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Self-powered soft robot in the Mariana Trench
A free-swimming soft robot inspired by deep-sea creatures, with artificial muscle, power and control electronics spread across a polymer matrix, successfully adapts to high pressure and operates in the deep ocean.
- Guorui Li
- , Xiangping Chen
- & Wei Yang
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Strong tough hydrogels via the synergy of freeze-casting and salting out
A strategy that combines freeze-casting and salting-out treatments produces strong, tough, stretchable and fatigue-resistant poly(vinyl alcohol) hydrogels.
- Mutian Hua
- , Shuwang Wu
- & Ximin He
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Facile route to bulk ultrafine-grain steels for high strength and ductility
Bulk ultrafine-grained steel is prepared by an approach that involves the rapid production of coherent, disordered nanoprecipitates, which restrict grain growth but do not interfere with twinning or dislocation motion, resulting in high strength and ductility.
- Junheng Gao
- , Suihe Jiang
- & W. Mark Rainforth
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Article |
A reprogrammable mechanical metamaterial with stable memory
A reprogrammable mechanical metamaterial constructed of bistable unit cells that can be switched independently and reversibly between two stable states with distinct mechanical properties using magnetic actuation is demonstrated.
- Tian Chen
- , Mark Pauly
- & Pedro M. Reis
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Article |
Strain-hardening and suppression of shear-banding in rejuvenated bulk metallic glass
Bulk metallic glasses can acquire the ability to strain-harden through a mechanical rejuvenation treatment at room temperature that retains their non-crystalline structure.
- J. Pan
- , Yu. P. Ivanov
- & A. L. Greer
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Letter |
Tuning element distribution, structure and properties by composition in high-entropy alloys
In high-entropy alloys, atomic-resolution chemical mapping shows that swapping some of the atoms for larger, more electronegative elements results in atomic-scale modulations that produce higher yield strength, excellent strain hardening and ductility.
- Qingqing Ding
- , Yin Zhang
- & Qian Yu
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Damage-tolerant architected materials inspired by crystal microstructure
Inspired by the enhanced mechanical strength of microstructured metals, damage-tolerant architected materials are developed in which the internal structure is granular, with different regions having different lattice orientations.
- Minh-Son Pham
- , Chen Liu
- & Jedsada Lertthanasarn
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Perspective |
Structural superlubricity and ultralow friction across the length scales
The phenomenon of ultralow friction between sliding incommensurate crystal surfaces—structural superlubricity—is examined, and the challenges and opportunities involved in its extension to the macroscale are assessed.
- Oded Hod
- , Ernst Meyer
- & Michael Urbakh
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Letter |
Enhanced strength and ductility in a high-entropy alloy via ordered oxygen complexes
Ordered oxygen complexes in high-entropy alloys enhance both strength and ductility in these compositionally complex solid solutions.
- Zhifeng Lei
- , Xiongjun Liu
- & Zhaoping Lu
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Letter |
Three-dimensional printing of hierarchical liquid-crystal-polymer structures
3D printing of liquid-crystal polymers can create lightweight hierarchical structures with very high stiffness and toughness.
- Silvan Gantenbein
- , Kunal Masania
- & André R. Studart
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Letter |
Topological negative refraction of surface acoustic waves in a Weyl phononic crystal
Sound waves in a specially designed crystal undergo ‘topologically protected’ negative refraction, whereby no reflection is allowed, at certain facets of the crystal and positive refraction at others.
- Hailong He
- , Chunyin Qiu
- & Zhengyou Liu
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Letter |
Rapid energy-efficient manufacturing of polymers and composites via frontal polymerization
Frontal polymerization of dicyclopentadiene is used to generate thermoset polymers and composite materials with much lower energy requirements and cure times than are needed in conventional oven or autoclave curing approaches.
- Ian D. Robertson
- , Mostafa Yourdkhani
- & Scott R. White
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Letter |
Sterically controlled mechanochemistry under hydrostatic pressure
‘Molecular anvil’ molecules consisting of a compressible mechanophore and incompressible ligands react under hydrostatic pressure to produce elemental metal via an unexplored mechanism.
- Hao Yan
- , Fan Yang
- & Nicholas A. Melosh
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Letter |
Processing bulk natural wood into a high-performance structural material
A process is described for the transformation of bulk wood into a low-cost, strong, tough, lightweight structural material, by the partial removal of lignin and hemicellulose followed by hot-pressing to densify the natural wood.
- Jianwei Song
- , Chaoji Chen
- & Liangbing Hu
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Letter |
Granular materials flow like complex fluids
The relaxation dynamics of granular materials is more like that of complex fluids than that of thermal glass-forming systems, owing to the absence of the ‘cage effect’.
- Binquan Kou
- , Yixin Cao
- & Yujie Wang
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Letter |
History-independent cyclic response of nanotwinned metals
In copper components containing highly oriented nanotwins, correlated ‘necklace’ dislocations moving back and forth offer an unusually fatigue-resistant response to engineering stress.
- Qingsong Pan
- , Haofei Zhou
- & Lei Lu
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Letter |
Probing the limits of metal plasticity with molecular dynamics simulations
The limits of dislocation-mediated metal plasticity are studied by using in situ computational microscopy to reduce the enormous amount of data from fully dynamic atomistic simulations into a manageable form.
- Luis A. Zepeda-Ruiz
- , Alexander Stukowski
- & Vasily V. Bulatov
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Letter |
3D printing of high-strength aluminium alloys
Zirconium nanoparticles introduced into aluminium alloy powders control solidification during 3D printing, enabling the production of crack-free materials with strengths comparable to the corresponding wrought material.
- John H. Martin
- , Brennan D. Yahata
- & Tresa M. Pollock
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Letter |
Mimicking biological stress–strain behaviour with synthetic elastomers
A polymer code based on a triplet of parameters—network strand length, side-chain length and grafting density—enables materials to be designed with specific combinations of mechanical properties to mimic biological materials.
- Mohammad Vatankhah-Varnosfaderani
- , William F. M. Daniel
- & Sergei S. Sheiko
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Letter |
Ultrastrong steel via minimal lattice misfit and high-density nanoprecipitation
A method of producing superstrong yet ductile steels using cheaper and lighter alloying elements is described, based on minimization of the lattice misfit to achieve a maximal dispersion of nanoprecipitates, leading to ultimate precipitation strengthening.
- Suihe Jiang
- , Hui Wang
- & Zhaoping Lu