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| Open AccessThe collective photothermal effect of silver nanoparticles probed by a microbolometer
Due to their plasmonic properties, silver nanoparticles are promising across a vast range of applications, from physics instrumentation to biomedicine and environmental science. Here, the photon-to-heat conversion efficiency of individual nanoparticles is elucidated by designing and fabricating an ultra-sensitive bolometer with 26 pW power resolution.
- Hanliang Zhu
- , Evelína Gablech
- & Pavel Neuzil
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Article
| Open AccessActivation of telecom emitters in silicon upon ion implantation and ns pulsed laser annealing
Defected silicon has uses in optically active telecom emitters. Here, nanosecond pulsed laser annealing is demonstrated as a non-invasive, localized method to activate the defects in high-purity silicon substrates.
- Greta Andrini
- , Gabriele Zanelli
- & Jacopo Forneris
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Article
| Open AccessLocal tuning of Rydberg exciton energies in nanofabricated Cu2O pillars
Rydberg excitons in cuprous oxide feature giant optical nonlinearities that may be exploited in quantum applications if suitably confined. Here, the authors show how exciton confinement can be realised by focused-ion-beam etching of Cu2O crystals without noticeable degradation of excitonic properties.
- Anindya Sundar Paul
- , Sai Kiran Rajendran
- & Hamid Ohadi
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Article
| Open AccessQuantum simulation of an extended Dicke model with a magnetic solid
The Dicke model, describing the cooperative coupling of an ensemble of two-level atoms with a single-mode light field, has a rich phenomenology in quantum optics and quantum information, but its analytical or numerical solution is beyond current reach. Here, a solid-state quantum simulator of an extended Dicke model is achieved using ErFeO3 crystals, where terahertz spectroscopy and magnetocaloric effect measurements reveal an atomically ordered phase in addition to the expected superradiant and normal phases.
- Nicolas Marquez Peraca
- , Xinwei Li
- & Junichiro Kono
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Article
| Open AccessBand transport evidence in PEDOT:PSS films using broadband optical spectroscopy from terahertz to ultraviolet region
Hole-doped polymer PEDOT:PSS shows high conductivity but the carrier transport mechanism is not yet clarified. Here, broadband optical conductivity spectra are derived using terahertz time-domain spectroscopy and far-infrared to-ultraviolet reflection spectroscopy, demonstrating band transport of hole carriers.
- Zijing Guo
- , Tetsu Sato
- & Hiroshi Okamoto
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Article
| Open AccessDeeply subwavelength mid-infrared phase retardation with α-MoO3 flakes
Polarization rotation is key for modern optics but achieving it at mid-infrared frequencies is challenging and requires very thick phase retarders. Here, α-MoO3 flakes provide mid-infrared phase retardation and 90 degrees polarization rotation within one micrometer of material, a thickness ten times thinner than the operational wavelength.
- Michael T. Enders
- , Mitradeep Sarkar
- & Georgia T. Papadakis
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Article
| Open AccessPolarization superposition of room-temperature polariton condensation
Cavity polariton condensates are promising for room temperature quantum technologies, but realizing polaritonic qubit states remains challenging. Here, polarization superposition of polariton states and laser-induced polarization switching are observed in a perovskite microcavity at room temperature, suggesting a coupling between orthogonally polarized states that could enable polaritonic qubits.
- Yuta Moriyama
- , Takaya Inukai
- & Kenichi Yamashita
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Article
| Open AccessEnhanced luminescence efficiency in Eu-doped GaN superlattice structures revealed by terahertz emission spectroscopy
A superlattice structure in Eu-doped GaN is known to improve the power output of red LEDs, though the mechanism behind this needs to be further established. Here, terahertz emission spectroscopy is used to understand the role played by potential barriers and carrier confinement in determining power output.
- Fumikazu Murakami
- , Atsushi Takeo
- & Masayoshi Tonouchi
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Article
| Open AccessNeural network interatomic potential for laser-excited materials
Using machine learning to construct interatomic potentials when materials are not in their electronic ground state is challenging. Here, a neural network interatomic potential is constructed for laser-excited silicon, which extends first-principles accuracy to ultra-large length and time scales.
- Pascal Plettenberg
- , Bernd Bauerhenne
- & Martin E. Garcia
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Article
| Open AccessInvestigating the operation mechanism of light-emitting electrochemical cells through operando observations of spin states
Light-emitting electrochemical cells are next-generation light-emitting devices but the operation mechanism is still not well understood microscopically. Here, the operation mechanism of light-emitting electrochemical cells is microscopically investigated by operando observation of spin states.
- Junya Katsumata
- , Fumiya Osawa
- & Kazuhiro Marumoto
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Article
| Open AccessSelf-organized patterning on azo molecular glass film via optical near-field effect
Self-organized surface patterning is of great interest fundamentally and in applications. Here, a complex patterning behavior is observed on an azo molecular glass film with surface polystyrene microspheres upon circularly polarized laser irradiation.
- Zenan Wang
- , Hao Huang
- & Xiaogong Wang
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Review Article
| Open AccessDevelopment and challenges in perovskite scintillators for high-resolution imaging and timing applications
Scintillators are materials of great interest for versatile and fast radiation detection systems. This Review discusses recent advances and strategies to improve the light yield, decay time, and coincidence timing resolution of all-inorganic and hybrid organic-inorganic perovskite scintillators.
- Arie Wibowo
- , Md Abdul Kuddus Sheikh
- & Muhammad Danang Birowosuto
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Article
| Open AccessDynamic spatio-temporal control of naturally sourced soft photonic crystals
Controlling the dynamics of natural soft photonic systems is challenging due to difficulties in sourcing and stimulating them. Here, natural bovine tapetum is used to investigate soft biophotonic crystals and dynamically control their response, providing insight into the development of displays and dynamic light management.
- Giulia Guidetti
- , Chris Pirie
- & Fiorenzo G. Omenetto
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Article
| Open AccessWide-bandgap GaN-based watt-class photonic-crystal lasers
Short-wavelength lasers based on wide-bandgap GaN photonic crystals are promising for high-brightness illumination and materials processing. Here, the authors develop a nano-fabrication method for GaN/air photonic crystals, achieving high lasing operation performance in terms of output power, beam quality, and low threshold current.
- Kei Emoto
- , Tomoaki Koizumi
- & Susumu Noda
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Article
| Open AccessCoexistence of two types of short-range order in Si–Ge–Sn medium-entropy alloys
Short-range chemical ordering has emerged as a key feature for controlling the properties of high-entropy alloys. Here, ab initio calculations reveal that two types of short-range ordering exist in Si–Ge–Sn medium-entropy alloys, suggesting that multiple types of ordering could exist in a single alloy.
- Xiaochen Jin
- , Shunda Chen
- & Tianshu Li
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Article
| Open AccessDoped semiconducting polymer nanoantennas for tunable organic plasmonics
Optical nanoantennas based on organic plasmonics are promising for their higher degree of tunability over metallic nanostructures. Here, nanodisks of polythiophene-based semiconducting polymers provide nanooptical antennas with resonances that are tunable over a 1000 nm wavelength range and can be switched off or on by doping modulation.
- Akchheta Karki
- , Yu Yamashita
- & Magnus P. Jonsson
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Article
| Open AccessNanoscale light field imaging with graphene
Nanoscale light manipulation and characterization are essential in nano-optics, but conventional microscopy or indirect imaging methods are often limited by low resolution or invasive nature. Here, a non-destructive light-field imaging with ~20 nm resolution is realized by p-n junction photodetection in graphene controlled by gate voltage.
- Tongcheng Yu
- , Francisco Rodriguez
- & Alexander N. Grigorenko
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Article
| Open AccessStabilized director buckling patterns in nematic elastomers and their dynamic optical effects
Light diffusion effects in liquid crystals are important for security and lighting devices. Here, viewing angle dependent pearlescence and iridescence are reported in a nematic liquid crystal elastomer with a stabilized director buckling pattern, which can be controlled by deformation or temperature.
- Takuya Ohzono
- , Hiroyuki Minamikawa
- & Eugene M. Terentjev
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Article
| Open AccessControlling triplet–triplet upconversion and singlet-triplet annihilation in organic light-emitting diodes for injection lasing
Losses induced by triplet excitons are a major obstacle for electrically pumped organic lasers. Here, a combination of enhanced triplet-triplet upconversion and suppressed singlet-triplet annihilation is demonstrated as a route towards lasing in organic light emitting diodes.
- Atul Shukla
- , Monirul Hasan
- & Ebinazar B. Namdas
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Review Article
| Open AccessDesign principles and biological applications of red-emissive two-photon carbon dots
Carbon dots are suitable for a range of biological applications due to their unique physicochemical properties and biological behavior. This Review summarizes research related to the emerging field of red-emissive two-photon carbon dots for bioimaging, biosensing, and phototherapeutic applications.
- Pooria Lesani
- , Aina Hazeera Mohamad Hadi
- & Hala Zreiqat
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Article
| Open AccessHigh efficiency green InP quantum dot light-emitting diodes by balancing electron and hole mobility
Developing green-emitting InP quantum dot light-emitting diodes (QLED) is lagging behind their red and green counterparts. Here, green InP quantum dots are prepared and incorporated into a QLED so to promote hole transport and reduce electron mobility, resulting in a maximum quantum efficiency of 16.3 %.
- Wei-Chih Chao
- , Tzu-Hsuan Chiang
- & Pi-Tai Chou
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Article
| Open AccessA transparent waveguide chip for versatile total internal reflection fluorescence-based microscopy and nanoscopy
Total internal reflection fluorescence microscopy typically relies on opaque optical waveguides, compatible only with upright microscopes. Here, a versatile approach is reported that uses CMOS-compatible transparent chips, demonstrated for the imaging of synthetic and biological samples, including super-resolution applications.
- Anish Priyadarshi
- , Firehun Tsige Dullo
- & Ganapathy Senthil Murugan
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Article
| Open AccessEffect of chemically induced permittivity changes on the plasmonic properties of metal nanoparticles
Studying the bonding of organic molecules onto the surface of metal nanomaterials is important for understanding their plasmonic properties. Here, changes in the electron density of states at the metal-ligand interface of Ag nanoparticles are linked to variations in localized dipole moments and interface permittivity.
- Noboru Saito
- , Sou Ryuzaki
- & Kaoru Tamada
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Article
| Open AccessElectro-absorption modulation in GeSn alloys for wide-spectrum mid-infrared applications
Silicon-based electronic-photonic integrated circuits are promising for various applications, but their mid-infrared optical modulation is elusive. Here, tunable mid-infrared electro-absorption modulation, with broadband operation range >140 nm, is achieved in GeSn alloys on Si by controlling the Sn content.
- Yun-Da Hsieh
- , Jun-Han Lin
- & Guo-En Chang
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Article
| Open AccessHigh-resolution stereolithography using a static liquid constrained interface
Stiction between polymerized layers and the constraining solid interface during stereolithography limits resolution. Here, a static inert liquid is used as a constraining interface to mitigate stiction, enabling high resolution parts to be fabricated with feature sizes spanning tens to thousands of microns.
- Aftab A. Bhanvadia
- , Richard T. Farley
- & Toshikazu Nishida
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Article
| Open AccessDirected self-assembly of soft 3D photonic crystals for holograms with omnidirectional circular-polarization selectivity
Controlling the alignment of blue phase liquid crystals is challenging. Here, electric-field induced phase transitions are exploited to control the crystal orientation of blue phase I, and applied to the fabrication of holograms with omnidirectional circular-polarization selectivity.
- SeongYong Cho
- , Misaki Takahashi
- & Masanori Ozaki
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Article
| Open AccessDirect correlation of local fluence to single-pulse ultrashort laser ablated morphology
Describing the laser ablation process with reduction-free data is important for furthering its use in modern manufacturing. Here, fluence maps, correlating laser beam intensity and ablated depth at each point in a full two-dimensional space, provide a method to probe ablation morphology in cases of arbitrary beam and crater profiles.
- Haruyuki Sakurai
- , Kuniaki Konishi
- & Makoto Kuwata-Gonokami
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Article
| Open AccessStretchable micro-scale concentrator photovoltaic module with 15.4% efficiency for three-dimensional curved surfaces
The use of photovoltaic devices for energy harvesting in real-world applications requires that they are conformable to non-flat surfaces. Here, a micro-scale concentrator module shows 15.4% outdoor conversion efficiency and can stretch over curved 3D surfaces.
- Daisuke Sato
- , Taizo Masuda
- & Noboru Yamada
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Article
| Open AccessInteraction of edge exciton polaritons with engineered defects in the hyperbolic material Bi2Se3
Hyperbolic materials have unique optical properties such as negative refraction and highly directional polaritons, relevant in super-resolution imaging. Here, the topological insulator Bi2Se3 is shown to host hyperbolic edge-confined exciton polaritons that can be steered via engineered edge defects.
- Robin Lingstädt
- , Nahid Talebi
- & Peter A. van Aken
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Article
| Open AccessHigh responsivity in MoS2 phototransistors based on charge trapping HfO2 dielectrics
MoS2 is a promising two-dimensional material for optoelectronics. Here, MoS2 phototransistors with a dual-functioning HfO2 dielectric and charge-trapping layer achieve a responsivity of 1.1×106, due to an enhanced photogating effect from band edge alignment with oxygen vacancies.
- Roda Nur
- , Takashi Tsuchiya
- & Mitsuru Takenaka
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Article
| Open AccessEnhanced hole injection assisted by electric dipoles for efficient perovskite light-emitting diodes
Perovskite nanocrystals are promising for use in light emitting diodes, but improved hole injection is needed. Here, MoO3 is added as an electric dipole layer between hole injection and transport layers, achieving a current efficiency of 72.7cd/A in a green light emitting diode.
- Xiangtian Xiao
- , Kai Wang
- & Wallace C. H. Choy
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Article
| Open AccessLong-distance coupling and energy transfer between exciton states in magnetically controlled microcavities
Coupling of semiconductor quantum wells is governed by short-range interactions, and thus limited to distances of roughly 10 nm. Here, magnetically controlled energy transfer between quantum wells over a distance of 2.15 μm is achieved via polariton-mediated coupling.
- Maciej Ściesiek
- , Krzysztof Sawicki
- & Jan Suffczyński
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Article
| Open AccessConstraint-free wavelength conversion supported by giant optical refraction in a 3D perovskite supercrystal
In nonlinear optics, efficient frequency conversion typically requires phase-matching conditions, resulting in wavelength, polarization, and angular selectivity. Here, these constraints are overcome in a supercrystal with giant refraction index, allowing wide spectral and angular acceptance.
- Ludovica Falsi
- , Luca Tartara
- & Eugenio DelRe
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Article
| Open AccessTwo-photon photocurrent in InGaN/GaN nanowire intermediate band solar cells
Intermediate band solar cells have the ability to reach efficiencies similar to multijunction cells using a single semiconductor junction. Here, enhanced two-photon carrier generation is demonstrated on a silicon substrate in an InGaN/GaN quantum dot-in-nanowire heterostructure intermediate band solar cell.
- Ross Cheriton
- , Sharif M. Sadaf
- & Karin Hinzer
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Article
| Open AccessRydberg excitons in Cu2O microcrystals grown on a silicon platform
Cu2O is of great interest for its excitonic properties, yet challenges in its fabrication means that most experiments focus on naturally occurring samples. Here, scalable thermal oxidation is reported for the growth of Cu2O with low-defect content, allowing the observation of Rydberg excitons.
- Stephan Steinhauer
- , Marijn A. M. Versteegh
- & Val Zwiller
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Article
| Open AccessOptical modulation in Ge-rich SiGe waveguides in the mid-infrared wavelength range up to 11 µm
Mid-infrared optical modulators are important for detecting compounds in a wide range of applications, but are typically limited to short wavelengths. Now, a SiGe waveguide is used to fabricate an optical modulator that can reach wavelengths spanning 5.5 µm to 11 µm.
- Miguel Montesinos-Ballester
- , Vladyslav Vakarin
- & Delphine Marris-Morini
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Article
| Open AccessActive spatial control of terahertz plasmons in graphene
Controlling spatial conductivity in graphene is important for plasmonic devices, yet conductivity patterning typically changes the electromagnetic environment. Here, teraherz plasmons in graphene are confined to specific regions via a patterned zinc oxide gate, reducing electromagnetic coupling.
- Ngoc Han Tu
- , Katsumasa Yoshioka
- & Norio Kumada