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| Open AccessPhase-locked photon–electron interaction without a laser
Ultrafast photon–electron spectroscopy commonly requires a driving laser. Now, an inverse approach based on cathodoluminescence spectroscopy has allowed a compact solution to spectral interferometry inside an electron microscope, without a laser.
- Masoud Taleb
- , Mario Hentschel
- & Nahid Talebi
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Research Briefing |
Identifying the quantum fingerprint of plasmon polaritons
Coherent multidimensional spectroscopy with nanoscale spatial resolution was used to directly probe a plasmon polariton quantum wave packet. To reproduce these results an improved quantum model of photoemission was required, in which the coherent coupling between plasmons and electrons is accounted for with the plasmon excitations extending beyond a two-level model.
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Letter |
Detection of a plasmon-polariton quantum wave packet
Plasmonics allows precise engineering of light–matter interactions and is the driver behind many optical devices. The local observation of a plasmonic quantum wave packet is a step towards bringing these functionalities to the quantum regime.
- Sebastian Pres
- , Bernhard Huber
- & Tobias Brixner
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News & Views |
Down the RABBIT hole
Manipulating the chirality of electron vortices using attosecond metrology allows the clocking of continuum–continuum transitions, bringing the dream of time-resolved quantum physics a little closer.
- Jean Marcel Ngoko Djiokap
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Comment |
Controlling random lasing action
Random lasers made out of disordered media have a rich but often unpredictable laser light emission, in all directions and over many frequencies. Strategies for taming random lasing are emerging, which have the potential to deliver programmable lasers with unprecedented properties.
- Riccardo Sapienza
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Letter |
Excitonic insulator in a heterojunction moiré superlattice
Stacking monolayer WS2 on top of bilayer WSe2 creates conditions where electrons and holes can coexist in the structure. Their Coulomb interaction allows them to form bound pairs and hence an excitonic insulator state.
- Dongxue Chen
- , Zhen Lian
- & Su-Fei Shi
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Letter |
Ultrafast switching to an insulating-like metastable state by amplitudon excitation of a charge density wave
Ultrafast optical excitation of a charge density wave leads to the formation of a metastable gapped state that synchronizes with the underlying correlated phase.
- Naotaka Yoshikawa
- , Hiroki Suganuma
- & Ryo Shimano
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Letter |
Absolute 13C/12C isotope amount ratio for Vienna PeeDee Belemnite from infrared absorption spectroscopy
Isotope ratio measurements are complicated by the instabilities of composition in reference samples. Now a calibration-free method relying on infrared spectroscopy provides measurements that are traceable to International System of Units standards.
- Adam J. Fleisher
- , Hongming Yi
- & Joseph T. Hodges
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Article
| Open AccessEvidence for metastable photo-induced superconductivity in K3C60
Evidence for light-induced superconductivity in K3C60 was limited to optical methods due to the short lifetime of the phase. Extending the lifetime from picoseconds to nanoseconds now allows measurement of its negligible electrical resistance.
- M. Budden
- , T. Gebert
- & A. Cavalleri
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Letter
| Open AccessCharge radii of exotic potassium isotopes challenge nuclear theory and the magic character of N = 32
The charge radii of potassium isotopes up to 52K are measured, and show no sign of magicity at 32 neutrons as previously suggested in calcium. The observations are interpreted with coupled cluster and density functional theory calculations.
- Á. Koszorús
- , X. F. Yang
- & S. G. Wilkins
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News & Views |
Spin currents go nuclear
Generating pure spin currents is a necessary part of many spintronic devices. Now there is a new mechanism for doing this, utilizing nuclear spin waves.
- Claudia K. A. Mewes
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Review Article |
Antiferromagnetic opto-spintronics
An overview of how electromagnetic radiation can be used for probing and modification of the magnetic order in antiferromagnets, and possible future research directions.
- P. Němec
- , M. Fiebig
- & A. V. Kimel
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Letter |
Geodesy and metrology with a transportable optical clock
An atomic clock has been deployed on a field measurement campaign to determine the height of a mountain location 1,000 m above sea level, returning a value that is in good agreement with state-of-the-art geodesy.
- Jacopo Grotti
- , Silvio Koller
- & Davide Calonico
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News & Views |
Nuclear spins get a comb-over
A frequency comb technique used in NMR spectroscopy reveals the dynamics of the nuclear spin bath in self-assembled quantum dots.
- Jeroen Elzerman
- & Mark Buitelaar
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Letter |
Direct measurement of exciton valley coherence in monolayer WSe2
Coherent valley exciton dynamics are directly probed in a monolayer transition metal dichalcogenide, providing access to the valley coherence time and decoherence mechanisms — crucial for developing methods for manipulating the valley pseudospin.
- Kai Hao
- , Galan Moody
- & Xiaoqin Li
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News & Views |
Enlightened state
Determining the sequence of events following photon absorption by a molecule can be a surprisingly challenging task. An innovative use of time-resolved X-ray spectroscopy has revealed an important insight into the ultrafast excited-state dynamics of a well-known inorganic chromophore.
- James K. McCusker
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Letter |
Terahertz control of nanotip photoemission
Nanoscale metallic tips are a useful source of electrons for material characterization. It is now shown how terahertz radiation can provide precision control and enhancement of photoelectron emission from these sources. The approach can shape the spectrum of the electron pulse, which could pave the way to improvements in ultrafast electron diffraction and transmission electron microscopy.
- L. Wimmer
- , G. Herink
- & C. Ropers
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News & Views |
Combs grow bigger teeth
A combination of two Nobel ideas circumvents the trade-off between power and accuracy in ultraviolet spectroscopy.
- Scott A. Diddams
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Letter |
Ramsey-comb spectroscopy with intense ultrashort laser pulses
Frequency combs provide a broad series of well-calibrated spectral lines for highly precise metrology and spectroscopy, but this usually involves a trade-off between power and accuracy. A comb created by adjusting the time delay between two optical pulses now enables both. This so-called Ramsey comb could probe fundamental problems such as determining the size of the proton.
- Jonas Morgenweg
- , Itan Barmes
- & Kjeld S. E. Eikema
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Letter |
Sensing and atomic-scale structure analysis of single nuclear-spin clusters in diamond
Being able to sense nuclear spin dimers is an important next step towards single-molecule structural analysis from NMR measurements. Now the sensing of a single 13C–13C nuclear spin dimer near a nitrogen–vacancy centre in diamond is reported, together with a structural characterization at atomic-scale resolution.
- Fazhan Shi
- , Xi Kong
- & Jiangfeng Du
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Article |
Vibrational and electronic dynamics of nitrogen–vacancy centres in diamond revealed by two-dimensional ultrafast spectroscopy
Emerging sensing and quantum-information technologies based on nitrogen–vacancy centres in diamond require a better understanding of the relaxation mechanisms. A two-dimensional spectroscopy study provides information about the effects of the vibrational bath on the electronic dynamics.
- V. M. Huxter
- , T. A. A. Oliver
- & G. R. Fleming
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Letter |
Harnessing nuclear spin polarization fluctuations in a semiconductor nanowire
Ensembles of nuclear spins display thermal fluctuations—spin noise—that interfere with nuclear magnetic resonance measurements of samples below a threshold size. Experiments on nanowires show that by monitoring spin noise in real time and applying instantaneously adjusted radiofrequency pulses, spin polarization distributions that are narrower than the thermal distribution can be obtained.
- P. Peddibhotla
- , F. Xue
- & M. Poggio
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News & Views |
Long live the spin
A technique for protecting out-of-equilibrium nuclear spin states from thermalization while offering a route to converting them into observable NMR signal is an important contribution to a field that welcomes every bit of extra signal.
- Andreas Trabesinger
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Article |
Accessing long-lived nuclear singlet states between chemically equivalent spins without breaking symmetry
Short nuclear spin–lattice relaxation times have long been a challenge for magnetic resonance imaging. The alternative of using long-lived nuclear spin states has so far required symmetry breaking, but a method of controlling these states without breaking the symmetry of the spin system has now been demonstrated.
- Yesu Feng
- , Ryan M. Davis
- & Warren S. Warren
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Letter |
The origin and non-quasiparticle nature of Fermi arcs in Bi2Sr2CaCu2O8+δ
How and why Fermi arcs—disconnected segments of the Fermi surface—emerge in the pseudogap phase of cuprate superconductors is a mystery. A technique for analysing angle-resolved photoemission spectroscopy data that removes momentum broadening effects suggests these arcs do not reflect true Fermi surface states, which would explain why they do not form continuous loops.
- T. J. Reber
- , N. C. Plumb
- & D. S. Dessau